Packed bed sorption enhanced methane reforming on CaO/CuO/Al2O3(NiO) catalyst

Giuseppe Diglio; Piero Bareschino; Erasmo Mancusi; Francesco Pepe; Dawid Hanak; Vasilije Manovic

doi:10.1016/B978-0-444-64235-6.50243-6

Packed bed sorption enhanced methane reforming on CaO/CuO/Al₂O₃(NiO) catalyst

Giuseppe Diglio, Piero Bareschino, Erasmo Mancusi, Francesco Pepe, Dawid Hanak, Vasilije Manovic

Research output: Chapter in Book/Report/Conference proceeding › Chapter

1 Citation (Scopus)

Abstract

An autothermal sorption-enhanced steam methane reforming in a packed-bed reactor for production of high-purity hydrogen was studied by means of 1D numerical model. The reactor utilises a CaO/CuO/Al₂O₃(NiO) catalyst. This process is characterised by a number of challenges, such as the choice of the operating conditions to ensure both a production of high-purity H₂ stream and an autothermal sorbent regeneration stage. This paper addresses these challenges through numerical simulation. The results for the system cyclically operated in a packed-bed showed a methane conversion of 95%, and a hydrogen yield and selectivity around 3 mol_H2·mol_CH4 ^-1 and 90%, respectively.

Original language	English
Title of host publication	Computer Aided Chemical Engineering
Editors	Anton Friedl, Jiří J. Klemeš, Stefan Radl, Petar S. Varbanov, Thomas Wallek
Publisher	Elsevier
Pages	1389-1394
Number of pages	6
ISBN (Print)	9780444642356
DOIs	https://doi.org/10.1016/B978-0-444-64235-6.50243-6
Publication status	Published - 1 Jan 2018
Externally published	Yes

Publication series

Name	Computer Aided Chemical Engineering
Volume	43
ISSN (Print)	1570-7946

Bibliographical note

Publisher Copyright:
© 2018 Elsevier B.V.

Access to Document

10.1016/B978-0-444-64235-6.50243-6

Cite this

Diglio, G., Bareschino, P., Mancusi, E., Pepe, F., Hanak, D., & Manovic, V. (2018). Packed bed sorption enhanced methane reforming on CaO/CuO/Al₂O₃(NiO) catalyst. In A. Friedl, J. J. Klemeš, S. Radl, P. S. Varbanov, & T. Wallek (Eds.), Computer Aided Chemical Engineering (pp. 1389-1394). (Computer Aided Chemical Engineering; Vol. 43). Elsevier. https://doi.org/10.1016/B978-0-444-64235-6.50243-6

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abstract = "An autothermal sorption-enhanced steam methane reforming in a packed-bed reactor for production of high-purity hydrogen was studied by means of 1D numerical model. The reactor utilises a CaO/CuO/Al2O3(NiO) catalyst. This process is characterised by a number of challenges, such as the choice of the operating conditions to ensure both a production of high-purity H2 stream and an autothermal sorbent regeneration stage. This paper addresses these challenges through numerical simulation. The results for the system cyclically operated in a packed-bed showed a methane conversion of 95%, and a hydrogen yield and selectivity around 3 molH2·molCH4 -1 and 90%, respectively.",

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Diglio, G, Bareschino, P, Mancusi, E, Pepe, F, Hanak, D & Manovic, V 2018, Packed bed sorption enhanced methane reforming on CaO/CuO/Al₂O₃(NiO) catalyst. in A Friedl, JJ Klemeš, S Radl, PS Varbanov & T Wallek (eds), Computer Aided Chemical Engineering. Computer Aided Chemical Engineering, vol. 43, Elsevier, pp. 1389-1394. https://doi.org/10.1016/B978-0-444-64235-6.50243-6

Packed bed sorption enhanced methane reforming on CaO/CuO/Al₂O₃(NiO) catalyst. / Diglio, Giuseppe; Bareschino, Piero; Mancusi, Erasmo et al.
Computer Aided Chemical Engineering. ed. / Anton Friedl; Jiří J. Klemeš; Stefan Radl; Petar S. Varbanov; Thomas Wallek. Elsevier, 2018. p. 1389-1394 (Computer Aided Chemical Engineering; Vol. 43).

Research output: Chapter in Book/Report/Conference proceeding › Chapter

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T1 - Packed bed sorption enhanced methane reforming on CaO/CuO/Al2O3(NiO) catalyst

AU - Diglio, Giuseppe

AU - Bareschino, Piero

AU - Mancusi, Erasmo

AU - Pepe, Francesco

AU - Hanak, Dawid

AU - Manovic, Vasilije

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AB - An autothermal sorption-enhanced steam methane reforming in a packed-bed reactor for production of high-purity hydrogen was studied by means of 1D numerical model. The reactor utilises a CaO/CuO/Al2O3(NiO) catalyst. This process is characterised by a number of challenges, such as the choice of the operating conditions to ensure both a production of high-purity H2 stream and an autothermal sorbent regeneration stage. This paper addresses these challenges through numerical simulation. The results for the system cyclically operated in a packed-bed showed a methane conversion of 95%, and a hydrogen yield and selectivity around 3 molH2·molCH4 -1 and 90%, respectively.

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